I did leave that out, dang. The compression ratio would be good to know. Cranking compression is also good but can be effected by the cam a little bit.
This would be more “Next Step up” cam.
https://www.summitracing.com/parts/hrs-711451-08/make/plymouth
If you have a few bucks, spring for a roller rocker set at a 1.6 ratio in an effort to take advantage of the heads better flowing capabilities over the stock head. You’ll go to .539 from the .506 lift on a more accurate rocker.
Choice #2;
https://www.summitracing.com/parts/hrs-710461-10
This one for a few more rpm’s. It has a higher lifts and duration but works a 2800 converter better. Also a 1.5 to a 1.6 with this cam, you go from a .525 to .560 intake, .531 - .566 exhaust. With this cam, I’d call Howard’s or ask if summit could have the LSA adjusted to a 108 considering your cubic inch displacement.
Nether cam will be great with power brakes. A vacuum can for brakes is always a good idea.
I personally think you ether have to much tire or not enough gear ratio. 3.55’s would be my minimum gear (and that’s pushing it some) and the maximum tire diameter would be 26 - 26-1/2 inch with that gear.
With the above combo I mentioned, the rate of acceleration is fine but long lasting. With your 3.23’s on 28’s, it’ll take you a mile or more to get to the top end of the tachometer. You’ll probably be doing around a 150 mph.
Do you need to travel the Hwy?
If not, you would have a good response from 3.91 gears.