This topic is a good read, thanks to all the contributors. I'll be going through this next spring. My '70 Charger had 195-75-14's on it when I bought it in 1986, and upgrading to 255-60-15's in the rear and 205-70-14's in the front made a very noticeable difference. I now have Cooper Cobra 275-60-15's on 9" rims for the rear, 235-60-15's on 8" rims for the front, planned for next spring. That alone will help even more, but I have the Moog offset bushings for the UCA's ready to install. At that point, I'll probably lower the front end at least an inch, then get an alignment. This could be considered Phase 1 of the handling mods as all of this is pretty affordable compared to the more radical, non-stock suspension upgrades.
Like Jamie from DDG says, these cars handle pretty good with the original torsion bar system, but some modern improvements make a big difference. I will probably consider fast-ratio Pitman & Idler arms for Phase 2, but that'll be a ways down the road.