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You have it backwardsI will tell you my experience put a bigger water pump pulley on it to increase the speed of the water pump. I had a customer we built a 512 stroker on pump gas, for a 4x4 truck and he wanted a serpentine belt system. The engine ran hot, swapped out radiators, high flow pumps, even took the heads back off and opened up the coolant holes in the head and block, changed to a bigger pulley problem solved. just use a stock A/C water pump. From your picture the pulley looks small to me.
To increase the RPM of your driven pulley, you can either increase the motor RPM or decrease the diameter of the driven pulley.